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The method of sensitive detection of ultraviolet (UV) radiation using integration of Cesium-Lead-Bromide perovskitebased nanocolloids with silicon avalanche photodiodes (APDs) was investigated. The perovskite nanoparticles (NPs) were synthesized using the sonication method with a conventional ultrasonic cleaning bath. The synthesis resulted in perovskite NPs in the form supercrystals of 200-nm diameter. The NPs being pumped with a 372-nm UV laser produced visible photoluminescence (PL) with a spectral peak at 514 nm. Integration of the perovskite nanocolloid with a silicon APD resulted in the increase of APD’s sensitivity to UV by ~7.6 dB. Degradation of the response of the perovskite-APD system to pulsed UV radiation at high frequencies was thus mainly due to the time delay in the APD (100-kHz cut-off frequency) rather than relaxation of the PL. Composition, crystalline structure, and UV-excited PL of two oxysulfide phosphors doped with Terbium (Y2O2S:Tb and Gd2O2S:Tb) were investigated with the view of their potential use in combination with silicon APDs for sensitive detection of x-ray radiation. Both phosphors contained oxide impurities Y2O3 and Gd2O3, respectively, partially reducing their x-ray scintillation capability. The obtained results might be useful for the applications in the field of sensitive detection of short wavelength (UV and x-ray) radiation.
(2024) Published by SPIE. Downloading of the abstract is permitted for personal use only.
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Darayas N. Patel, Sergey S. Sarkisov, Abdalla M. Darwish, Kelly Whyte, Sabrina Collins, Crystal Smith, "Sensitive detection of short wavelength radiation with spectrum down-converting nanoparticles," Proc. SPIE 12882, Optical Components and Materials XXI, 128820Q (8 March 2024); https://doi.org/10.1117/12.2690307